SVIBOR - Project code: 1-07-064

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Project code: 1-07-064


NATURAL ISOTOPES H-3, C-14, Th/U AND IONIZATION IN GASES


Main researcher: SRDOČ, DUŠAN (44284)



Assistants
Type of research: basic
Duration from: 01/01/91. to 12/31/95.

Papers on project (total): 77
Papers on project quoted in Current Contents: 21
Institution name: Institut "Ruđer Bošković", Zagreb (98)
Department/Institute: Department of Physics - Division for Experimental Physics
Address: 10001 Zagreb, P.p.1016, Bijenička 54
City: 10000 - Zagreb, Croatia
Communication
Phone: 385 (0)1 425 809
Fax: 385 (0)1 434 467
Fax: 385 (0)1 425 497
E-mail: obelic@olimp.irb.hr
E-mail: horvatin@olimp.irb.hr
E-mail: krajcar@olimp.irb.hr

Summary: Measurements of the specific activity of cosmogenic radionuclides (tritium, H-3 and radiocarbon, C-14) and radionuclides of uranium series were enabled in the last thirty years by the development of the measuring techniques. By C-14 dating method the ages of numerous archaeological, palaeontological and geological samples were determined. Hydrological characteristics (the mean residence time, recent infiltration, recharge area) of water-bearing layers of geothermal waters in NW Croatia and groundwaters in E Croatia were determined by isotopic methods (H-2, H-3, C-13, C-14, O-18). Geochronology of quaternary deposits, especially in karst regions in numerous speleological and travertine findings was determined. Cave formation and travertine deposits were dated by C-14 method up to 40000 years and by isotopes from uranium series (U-234/U-238, Th-230/U-234) up to 400000 years. The process of carbonate precipitation in freshwater has been studied by physico-chemical, isotopic and biological measurements. Measurements of C-14 and H-3 in the atmosphere, biosphere and hydrosphere have been applied in ecological studies. These characteristic applications of measurement of low specific activity were enabled by fundamental researches in the field of detection of ionizing radiation. The most important quantities studied in this project are the mean energy required to form an ion pair (W) in pure gases and gas mixtures, statistical fluctuations of the number of formed ion pairs (the Fano factor F) and charge multiplication in detectors. Theoretical study of interaction of electrons with atomic and molecular gases has been extended to subexcitation and thermal electrons.

Keywords: radioactive isotopes, H-3 (tritium), C-14 (radiocarbon), radiocarbon dating, stable isotopes, H-2, C-13, O-18, Th-230/U-234 dating, archaeology, hydrogeology, geochronology, aquatic chemistry, ionizing radiation, mean energy to form an ion pair (W), gas mixtures, electron degradation, electron thermalization

Research goals: The activity in the Laboratory was directed into two scientific fields: ISOTOPIC INVESTIGATIONS: Isotopic composition of surface and groundwater compared with the isotopic composition of precipitation gives important information about water movement: mean residence time of water in aquifers, the catchment area and the mixing ratio of groundwaters with surface waters. The data obtained have a significant application in hydrological investigations, contamination of surface and groundwaters and in investigation of precipitation processes of carbonates in karst waters. Measurement of the C-14 activity in various geological samples (carbonate sediments as speleothems, tufa and lake deposits) give important information about the age of geological formations in Holocene. Measurements of the concentration of isotopes C-14 and Th-230/U-234, as well as O-18, in carbonate sediments give a significant contribution to the study of palaeoclimatic conditions of the formation of quaternary depostis. Dating of archaeological samples of organic origin (bones, wood, charcoal, linen) is one of basic applications of radiocarbon method. The C-14 activity in the atmosphere and biosphere is systematically measured in order to determine environmental contamination. IONIZATION PROCESSES IN GASES: Exact knowledge of W values, the mean energy required to form an ion pair, is important in various applications of ionizing radiation, as well as in theoretical investigations. One of the goals of this project is to assess critically the existing W and F values for various ionizing particles in a variety of gases with an emphasis on gas mixtures. The aim of the experimental investigation of ionization in gases is to determine dependence of W and F values on the mixture parameters and the conditions in the proportional counter, as well as to define the experimental conditions that result in the best energy resolution. The goal of theoretical studies of electron degradation process in various energy regions is to define some fundamental principles underlying the degradation process in various gases and gas mixtures. These principles can be useful for application in plasma physics and radiation detection development.


COOPERATION - PROJECTS


  1. Name of project: CI1/900589 Application of Analytical Methods in Archaeology
    Name of institution: Commission of the European Communities, DG XII G3, SDME R2/144
    City: 1049 - Bruxelles, Belgija

  2. Name of project: JF-802/NSF Total Ionization Yield, the Fano Factors and Stochastic Distribution of Ions in Gases of Radiological Interest
    Name of institution: National Science Foundation (US-Yugoslav Joint Board for Scientific Research)
    City: DC - Washington, SAD

  3. Name of project: JF-800/NSF Study of Origin and Diagenesis of Travertine Deposits
    Name of institution: National Science Foundation (US-Yugoslav Joint Board for Scientific Research)
    City: DC - Washington, SAD

  4. Name of project: JF-839/NSF The Role of Biota in the Precipitation of Calcium Carbonate in Freshwater
    Name of institution: National Science Foundation (US-Yugoslav Joint Board for Scientific Research)
    City: DC - Washington, SAD

  5. Name of project: 5293/RB Total Ionization Yield for Low Energy Photons and Electrons Absorbed in Polyatomic Gases and Tissue-equivalent Gas Mixtures
    Name of institution: International Atomic Energy Agency
    City: 1400 - Beč, Austrija


COOPERATION - INSTITUTIONS


  1. Name of institution: Centro ricerca applicata e documentazione
    Type of institution: Institution whose primary activities ar
    Type of cooperation: Systematic exchange of information
    City: 33100 - Udine, Italija

  2. Name of institution: Inštitut Jožef Stefan
    Type of institution: State institute
    Type of cooperation: Systematic exchange of information
    City: 61000 - Ljubljana, Slovenija

  3. Name of institution: Filozofski fakultet Sveučilišta u Zagrebu
    Type of institution: University/Faculty
    Type of cooperation: Systematic exchange of information
    City: 10000 - Zagreb, Croatia

  4. Name of institution: Znanstvenoistraživački centar Hrvatske akademije znanosti i umjetnosti
    Type of institution: Other
    Type of cooperation: Systematic exchange of information
    City: 10000 - Zagreb, Croatia

  5. Name of institution: Institute of Isotopes of the Hungarian Academy of Sciences
    Type of institution: Other
    Type of cooperation: Systematic exchange of experts
    City: 1525 - Budapest, Mađarska

  6. Name of institution: International Atomic Energy Agency
    Type of institution: International organization
    Type of cooperation: Systematic exchange of information
    City: 1400 - Beč, Austrija

  7. Name of institution: Argonne National Laboratory
    Type of institution: State institute
    Type of cooperation: Joint publishing of scientific papers
    City: 60439 - Argonne, Illinois, SAD

  8. Name of institution: Physikalisch-Technische Bundesanstalt
    Type of institution: State institute
    Type of cooperation: Systematic exchange of experts
    City: 38116 - Braunschweig, Njemačka

  9. Name of institution: University of Glasgow
    Type of institution: University/Faculty
    Type of cooperation: Systematic exchange of information
    City: Glasgow, Scotland, Velika Britanija

  10. Name of institution: Universitat Autonoma de Barcelona - Department de Geologia, Unitat de cristal.lografia
    Type of institution: University/Faculty
    Type of cooperation: Systematic exchange of experts
    City: 08193 - Bellaterra/Barcelona, Spanjolska

  11. Name of institution: University of Texas
    Type of institution: University/Faculty
    Type of cooperation: Joint project
    City: Houston, Texas, SAD

  12. Name of institution: Geološki institut Zagreb
    Type of institution: State institute
    Type of cooperation: Systematic exchange of information
    City: 10000 - Zagreb, Croatia

  13. Name of institution: INA - Geološki konzalting
    Type of institution: Economical/Production
    Type of cooperation: Occasional exchange of information
    City: 10000 - Zagreb, Croatia

  14. Name of institution: Geološki fakultet, Zagreb
    Type of institution: University/Faculty
    Type of cooperation: Systematic exchange of information
    City: 10000 - Zagreb, Croatia

  15. Name of institution: Geološki zavod Ljubljana
    Type of institution: State institute
    Type of cooperation: Systematic exchange of information
    City: 61000 - Ljubljana, Slovenija

  16. Name of institution: University of Bern - Institute of Physics
    Type of institution: University/Faculty
    Type of cooperation: Systematic exchange of experts
    City: Bern, Švicarska

  17. Name of institution: University of Bern - Geological Institute
    Type of institution: University/Faculty
    Type of cooperation: Systematic exchange of information
    City: Bern, Švicarska

  18. Name of institution: Brookhaven National Laboratory
    Type of institution: State institute
    Type of cooperation: Joint publishing of scientific papers
    City: Upton, Long Island, New York, USA

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Last update: 09/25/95
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